Rheological characterisation and modelling of a glass mat reinforced thermoplastic for the simulation of compression moulding

Rheological characterisation and modelling of a glass mat reinforced thermoplastic for the simulation of compression moulding

ALTHAUS Philipp, WESTER Hendrik, ROSENBUSCH Daniel, BEHRENS Bernd-Arno

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Abstract. The use of hybrid components in the automotive industry is steadily increasing due to their lightweight potential. By combining fibre-reinforced plastics with metallic materials, high-strength components with lower weight than monolithic metal parts can be realised. The overall aim of the project “HyFiVe” is to exploit this potential for electric vehicles by developing a scaled battery housing structure made of a glass mat reinforced thermoplastic (GMT) paired with unidirectional reinforced (UD) tapes and a metallic reinforcement frame. The GMT is formed by compression moulding and serves as the base of the battery housing structure. Numerical simulation is an efficient tool for process design that can determine a suitable process window and reduce experimental trial-and-error tests. Particularly, realistic modelling of the GMT flow behaviour is essential for reliable simulation results. In this contribution, the rheological properties of a GMT consisting of a polyamide 6 (PA6) matrix with 30% glass fibre reinforcement were determined. Isothermal compression tests were carried out with a parallel plate rheometer at different temperatures and varying squeeze rates. The squeeze force and punch displacement were evaluated to determine the rheological data of the GMT. Two methods for the modeling of the flow behaviour were considered. At first, pure shear flow was assumed and the viscosity was modelled as a function of the shear rate by means of a power-law. Secondly, a pure biaxial extension was assumed and the true stress was modelled in dependence of true strain and strain rate. Subsequently, for a verification of the material models, the compression tests were simulated in ABAQUS using the Coupled Eulerian-Lagrange (CEL) approach and the results were compared to the experiments.

Keywords
Glass Mat Reinforced Thermoplastic, Material Characterisation, Squeeze Flow

Published online 4/24/2024, 11 pages
Copyright © 2024 by the author(s)
Published under license by Materials Research Forum LLC., Millersville PA, USA

Citation: ALTHAUS Philipp, WESTER Hendrik, ROSENBUSCH Daniel, BEHRENS Bernd-Arno, Rheological characterisation and modelling of a glass mat reinforced thermoplastic for the simulation of compression moulding, Materials Research Proceedings, Vol. 41, pp 411-421, 2024

DOI: https://doi.org/10.21741/9781644903131-46

The article was published as article 46 of the book Material Forming

Content from this work may be used under the terms of the Creative Commons Attribution 3.0 license. Any further distribution of this work must maintain attribution to the author(s) and the title of the work, journal citation and DOI.

References
[1] D.K. Rajak, D.D. Pagar, P.L. Menezes, E. Linul, Fiber-Reinforced Polymer Composites: Manufacturing, Properties, and Applications, Polymers 11 (2019). https://doi.org/10.3390/polym11101667
[2] K. Mocellin, P.-O. Bouchard, R. Bigot, T. Balan (Eds.), Proceedings of the 14th International Conference on the Technology of Plasticity – Current Trends in the Technology of Plasticity, Springer Nature Switzerland, Cham, 2024
[3] J. Karger-Kocsis, Polypropylene Structure, blends and Composites, Springer Netherlands, Dordrecht, 1995.
[4] B.-A. Behrens, S. Hübner, C. Bonk, F. Bohne, M. Micke-Camuz, Development of a Combined Process of Organic Sheet forming and GMT Compression Molding, Procedia Engineering 207 (2017) 101–106. https://doi.org/10.1016/j.proeng.2017.10.745
[5] J. Weichenhain, P. Althaus, S. Hübner, H. Wester, D. Rosenbusch, B.-A. Behrens, Investigation of a Compression Molding Process for the Variant Flexible Production of a GMT Battery Shell, in: B.-A. Behrens, A. Brosius, W.-G. Drossel, W. Hintze, S. Ihlenfeldt, P. Nyhuis (Eds.), Lecture Notes in Production Engineering, Production at the Leading Edge of Technology, Springer International Publishing, Cham, 2022, pp. 20–28.
[6] K.B. Thattaiparthasarthy, S. Pillay, U.K. Vaidya, Rheological characterization of long fiber thermoplastics – Effect of temperature, fiber length and weight fraction, Composites Part A: Applied Science and Manufacturing 40 (2009) 1515–1523. https://doi.org/10.1016/j.compositesa.2009.06.009
[7] J.R. Scott, Theory and application of the parallel-plate plastometer, Trans Inst Rubber Ind (1931) 169–186.
[8] G. Kotsikos, J.H. Bland, A.G. Gibson, H.W. Chandler, Squeeze flow testing of glass mat thermoplastic material, Composites Part A: Applied Science and Manufacturing 27 (1996) 1195–1200. https://doi.org/10.1016/1359-835X(96)00077-2
[9] S. Lee, D. Shin, G. Kim, W. Ji, Numerical model for compression molding process of hybridly laminated thermoplastic composites based on anisotropic rheology, Composites Part C: Open Access 7 (2022) 100215. https://doi.org/10.1016/j.jcomc.2021.100215
[10] M.A. Dweib, C.M.Ó. Brádaigh, Anisotropic modeling of isothermal squeezing flow of Glass-Mat reinforced thermoplastics (GMT), Polym Compos 19 (1998) 588–599. https://doi.org/10.1002/pc.10132
[11] D. Dörr, N. Singh-Heer, R.C. Gergely, L. Schreyer, F. Henning, A.G. Straatman, A. Hrymak, Rheological characterization and macroscopic modeling and simulation of the molding process of a PA6 Glass Mat Thermoplastic (GMT), Composites Part A: Applied Science and Manufacturing 176 (2024) 107780.
[12] C.-T. Huang, L.-J. Chen, T.-Y. Chien, Investigation of the Viscoelastic Behavior Variation of Glass Mat Thermoplastics (GMT) in Compression Molding, Polymers 11 (2019). https://doi.org/10.3390/polym11020335
[13] B.-A. Behrens, F. Bohne, R. Lorenz, H. Arndt, S. Hübner, M. Micke-Camuz, Numerical and Experimental Investigation of GMT Compression Molding and Fiber Displacement of UD-Tape Inserts, Procedia Manufacturing 47 (2020) 11–16. https://doi.org/10.1016/j.promfg.2020.04.109
[14] K. Dröder, B.-A. Behrens, F. Bohne, A. Chugreev, H. Schulze, B. Wonnenberg, Numerical and Experimental Investigation of Thermoplastics in Multi-Axis Forming Processes, Procedia CIRP 85 (2019) 96–101. https://doi.org/10.1016/j.procir.2019.09.024